Tomáš Mančal / Teaching / Nonlinear Optical Spectroscopy / Non-Linear Optical Spectroscopy / Introduction to Non-Linear Optical Spectroscopy /

12 - Construction of spectroscopy with simultaneous time and frequency resolutions

Details of the pump-probe detection scheme and its generalization to two non-colinear pump pulses. The idea of a generalized susceptibility for the probe pulse gets scrutinized and found valid under relatively general conditions. Constructing spectrum from complex lineshapes and the definition of a coherent two-dimensional (2D) spectra, which could provide a simultaneous high resolution in time and frequency. Basic properties of 2D spectrum.

Attachment: Lecture_11_part_1.pdf