Tomáš Mančal / Teaching / Nonlinear Optical Spectroscopy / Non-Linear Optical Spectroscopy / Introduction to Non-Linear Optical Spectroscopy /

13 - Two-dimensional Cohetent Fourier-transformed Spectroscopy

Summary of the expected properties of 2D spectrum introduced earlier. Geometric and temporal arrangements of the pulses in the 2D experiment. Detection of the complex non-linear signal and determination of its unknown phase factor. Example spectrum of a donor-acceptor system exhibiting energy transfer and no excited state delocalization. Complete discussion of the Liouville pathways composing the non-linear signal. Placement of the contribution of the individual Liouville pathways into a 2D spectrum.

Attachment: Lecture_12_part_1.pdf